Microscopic and continuum descriptions of Janus motor fluid flow felds

Microscopic and continuum descriptions of Janus motor fluid flow felds

Publication Type:

Journal Article

Source:

Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Royal Society of London, Volume 374, Number 2080 (2016)

URL:

https://www.scopus.com/inward/record.uri?eid=2-s2.0-84992017375&doi=10.1098%2frsta.2016.0140&partnerID=40&md5=ec8e36ad497d2daf978bc4f07c0c0539

Keywords:

active matter, Catalyst activity, Chemical, chemical model, chemistry, Computer Simulation, Concentration gradients, Continuum description, Continuum mechanics, diffusiophoresis, Energy Transfer, Flow of fluids, Fluid dynamics, Mechanical, mechanical stress, Microfluidics, Microscopic simulation, Models, Motion, Multi-scale modelling, nanoparticle, Nanoparticles, Naturally occurring, procedures, Spherical geometries, Stress, ultrastructure, Velocity

Abstract:

Active media, whose constituents are able to move autonomously, display novel features that differ from those of equilibrium systems. In addition to naturally occurring active systems such as populations of swimming bacteria, active systems of synthetic selfpropelled nanomotors have been developed. These synthetic systems are interesting because of their potential applications in a variety of fields. Janus particles, synthetic motors of spherical geometry with one hemisphere that catalyses the conversion of fuel to product and one non-catalytic hemisphere, can propel themselves in solution by self-diffusiophoresis. In this mechanism, the concentration gradient generated by the asymmetric catalytic activity leads to a force on the motor that induces fluid flows in the surrounding medium. These fluid flows are studied in detail through microscopic simulations of Janus motor motion and continuum theory. It is shown that continuum theory is able to capture many, but not all, features of the dynamics of the Janus motor and the velocity fields of the fluid. This article is part of the themed issue 'Multiscale modelling at the physics-chemistry-biology interface'. © 2016 The Author(s) Published by the Royal Society. All rights reserved.

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